Polímeros: Ciência e Tecnologia
https://revistapolimeros.org.br/article/doi/10.1590/0104-1428.20230022
Polímeros: Ciência e Tecnologia
Original Article

Cellulose fiber network as reinforcement of thermoplastic paraffin films

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The incorporation of natural fibers into polymer matrices poses challenges due to physicochemical incompatibility, which is typically addressed through precursor modification or the use of compatibilizers. Here, we introduce a novel type of composite that overcomes this challenge by utilizing a network of fine, porous cellulosic sheets inter-diffused with a commercial paraffin films. This approach physically adheres the fiber network to the matrix, preserving its structure. Microscopy images confirm the formation of the proposed microstructure, and mechanical testing reveals a gradual increase in modulus and strength with the incorporation of cellulose. The maximum incorporation achieved was 7.6% (w/w) of cellulosic fibers, resulting in a 167% increase (1.67 times improved) in composite stiffness. Moreover, these composites exhibit ductility, with an average deformation of 410 ± 38%, corresponding to 20% reduction in relation to pure matrix. Our findings demonstrate the potential of this approach for developing sustainable materials with improved mechanical properties.

 

 

natural fibers, composites, network reinforcement, paper, polymer matrices

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